I don't have any chalices, but have had both red & green Emeralds and Sally lightfoot crabs in my MD as well as all the common hermit varieties. IMO they (larger crab types) cover a niche in the CUC that neither hermits or snails fill. Mine are mostly noctural, but have never messed with any of my corals (mostly Z&Ps, but some digitata, ORA deepwater SPS, GSP, Leathers, Shrooms, etc...
Bouncing off of Harry's comments, I have had hermits attack and kill snails, but have never "witnessed" a larger type crab do it. Plus, none of mine have ever exceeded 2" (body width) in size. Looks like mixed reviews here and chalice's are an expensive coral to experiment with. Not sure what to tell ya.