Yes. The combination of really, really low nutrients, high lighting and high alkalinity is really, really not good for acros. Keep in mind, however, that if you have substantial algae in the tank, you might get very low nutrient readings. It's still not a good thing, but there's a difference between a nearly sterile tank with no algae growth to speak of and very low nutrients and one that's a little "dirty" with substantial algae and low nutrient readings.
After reading through these 6 pages, I'd say that you've nailed this with the help of Crustaceon. Generally speaking, dosing is required for an acro tank, whether using 2-part or a calcium reactor. Most of that's not the actual consumption of alkalinity and calcium, it's maintaining constant levels for months/years on end.
You mentioned a couple of pages back that you were going to go to weekly alk/calcium testing. I'd suggest that for the moment while you're hand dosing and getting the tank back on track, you do alk testing at least once every 2 days. Alkalinity stability is that important to an acro tank.
Finally, you mentioned feeding more and/or adding a 5th fish to boost your nitrate/phosphate numbers. That's certainly a possibility, but have you considered simply adding coral foods, such as ReefRoids, Oyster Feast, or something similar?