Actually,
those numbers are all fairly terrible, which is actually good. They are still relatively balanced, just very low due to lack of maintenance.
A must-read for your situation:
When Do Calcium and Alkalinity Demand Not Exactly Balance? by Randy Holmes-Farley - Reefkeeping.com
You should, however, stop adjusting alkalinity by itself immediately.
Adjustment in a balanced way is the only correct way in your case.
Ordinarily, I would recommend significant water changes with a well-fortified salt (e.g. Reef Crystals) combined with a balanced additive like limewater (kalkwasser).
Two-part also works, and since you started with the alkalinity part, I would recommend you just add the balanced proportions of Ca and Mg that match the alk you've already added (see the Reef Chemistry Calculator), and proceed from there.
If you stay with two-part, I would adjust your Mg up first - prevents Ca+alk precipitation and helps you get more accurate Ca and alk test numbers for your final adjustments. Follow that with 1/3 to 1/2 doses of Ca and alkalinity, followed by retesting on all three parameters. Followed by additional doses as needed. (Same advice should be in the Reef Chemistry Calculator when you are computing your adjustment doses.)
Keep me posted!
-Matt